#6538. Optimization of Monomer Molecular Structure for Polymer Electrodes Fabricated through in-situ Electro-Polymerization Strategy

March 2027publication date
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Journal’s subject area:
Chemical Engineering (all);
Energy (all);
Materials Science (all);
Environmental Chemistry;
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Abstract:
In-situ electro-polymerization of redox-active monomers has been proved to be a novel and facile strategy to prepare polymer electrodes with superior electrochemical performance. The monomer molecular structure would have a profound impact on electro-polymerization behavior and thus electrochemical performance. However, this impact is poorly understood and has barely been investigated yet. Herein, three carbazole-based monomers, 9-phenylcarbazole (CB), 1,4-bis(carbazol-9-yl)benzene (DCB), and 2,6-bis(carbazol-9-yl)naphthalene (DCN), were applied to study the above issue systematically and achieve excellent long cycle performance. The monomers were rationally designed with different polymerizable sites and solubilities.
Keywords:
electro-polymerization; energy storage; lithium-ion batteries; polymer electrodes; solubility

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